Electron screening length identifying circular dichroism of photoemission

Jiwon Jeon, J. D. Lee

Research output: Contribution to journalArticlepeer-review

Abstract

Circular dichroism angle-resolved photoemission spectroscopy (CD-ARPES) receives much attention due to a resolving power of topological and quantum geometrical nature of two-dimensional systems. We propose the Lippmann-Schwinger photoelectron final state, a scattering solution of the lattice model comprising screened short-range potentials at periodically arranged atomic sites, which characterizes the time-reversed low energy electron diffraction (LEED) state well enough to describe the final state effect entailed in CD-ARPES. We find that, through the final state effect, the electron screening length identifies CD-ARPES not only in the qualitative dichroic polarity but also in the quantitative dichroic strength in various graphene systems like the monolayer graphene, the AA-stacking bilayer graphene, and the twisted bilayer graphene especially in a unified fashion. This finding reveals an interplay between electron screening and circular dichroism and enables to extend the spectroscopic expertise of CD-ARPES to a direct probe of the electron screening.

Original languageEnglish
Article number147439
JournalJournal of Electron Spectroscopy and Related Phenomena
Volume273
DOIs
StatePublished - Jun 2024

Bibliographical note

Publisher Copyright:
© 2024 Elsevier B.V.

Keywords

  • Circular dichroism angle-resolved photoemission spectroscopy
  • Electron screening
  • Final state effect
  • Graphene materials
  • Lippmann-Schwinger final state

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